Alessia Romani

Design & Engineering Research

Recycled polycarbonate and polycarbonate/acrylonitrile butadiene styrene feedstocks for circular economy product applications with fused granular fabrication-based additive manufacturing


Journal article


Alessia Romani, Marinella Levi, Joshua M. Pearce*
Sustainable Materials and Technologies, vol. 38(e00730), 2023 Dec


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APA   Click to copy
Romani, A., Levi, M., & Pearce*, J. M. (2023). Recycled polycarbonate and polycarbonate/acrylonitrile butadiene styrene feedstocks for circular economy product applications with fused granular fabrication-based additive manufacturing. Sustainable Materials and Technologies, 38(e00730). https://doi.org/10.1016/j.susmat.2023.e00730


Chicago/Turabian   Click to copy
Romani, Alessia, Marinella Levi, and Joshua M. Pearce*. “Recycled Polycarbonate and Polycarbonate/Acrylonitrile Butadiene Styrene Feedstocks for Circular Economy Product Applications with Fused Granular Fabrication-Based Additive Manufacturing.” Sustainable Materials and Technologies 38, no. e00730 (December 2023).


MLA   Click to copy
Romani, Alessia, et al. “Recycled Polycarbonate and Polycarbonate/Acrylonitrile Butadiene Styrene Feedstocks for Circular Economy Product Applications with Fused Granular Fabrication-Based Additive Manufacturing.” Sustainable Materials and Technologies, vol. 38, no. e00730, Dec. 2023, doi:10.1016/j.susmat.2023.e00730.


BibTeX   Click to copy

@article{alessia2023a,
  title = {Recycled polycarbonate and polycarbonate/acrylonitrile butadiene styrene feedstocks for circular economy product applications with fused granular fabrication-based additive manufacturing},
  year = {2023},
  month = dec,
  issue = {e00730},
  journal = {Sustainable Materials and Technologies},
  volume = {38},
  doi = {10.1016/j.susmat.2023.e00730},
  author = {Romani, Alessia and Levi, Marinella and Pearce*, Joshua M.},
  month_numeric = {12}
}

Abstract

Distributed recycling and additive manufacturing (DRAM) holds enormous promise for enabling a circular economy. Most DRAM studies have focused on single thermoplastic waste stream. This study takes three paths forward from the previous literature: 1) expanding DRAM into high-performance polycarbonate/ acrylonitrile butadiene styrene (PC/ABS) blends, 2) extending PC/ABS blend research into both recycled materials and into direct fused granular fabrication (FGF) 3-D printing and 3) demonstrating the potential of using recycled PC/ABS feedstocks for new applications in circular economy contexts. A commercial open source large-format FGF 3-D printer was modified and used to assess the different printability and accuracy of recycled PC and PC/ABS. The mechanical properties (tensile and impact) following the ASTM D638 and D6110–18 standards were quantified. A weather simulation test (ASTM D5071–06) was performed to assess outdoor performance. Finally, two applications in sporting goods and furniture were demonstrated. In general, better printability was achieved with recycled PC/ABS compared to recycled PC, as well as good dimensional accuracy at printing speeds of 30 and 40 mm/s. Minimal qualitative differences and discoloration were visible on the samples after accelerated weather exposure, with results in accordance with the state-of-the-art. The rPC/ABS results from tensile tests show similar values to those of rPC for elastic modulus (2.1 ± 0.1 GPa), tensile strength (41.6 ± 6.3 MPA), and elongation at break (2.8 ± 0.9%), which are also comparable with previous studied virgin 3-D printed filaments. Similarly, impact energy (115.78 ± 24.40 kJ/m2) and resistance values (810.36 ± 165.77 J/m) are comparable in the two tested formulations, reaching similar results compared to FFF 3-D printed filaments, as well as virgin materials for injection molding. Finally, the two demonstration products in the sporting goods and furniture sectors were successfully fabricated with rPC/ABS, achieving complex patterns and good printing speeds for recycled feedstocks. It is concluded rPC/ABS blends represent a potential high-performance feedstock for DRAM, validating its use in direct FGF 3-D printing systems and potential applications for a circular economy. 1

Keywords

3-D printing // Recycling // Fused filament fabrication (FFF) // Fused granular fabrication (FGF) // Distributed recycling for additive manufacturing (DRAM) // Mechanical properties


Resources and links

  • 📑 Full text (publisher version) 2
  • 📝 Full text (preprint version) 3
  • 🛠️ OSF Repository (3D models and applications) 4
  • 🛠️ OSF Repository (3D models and modifications) 5



  1. Romani, A., Levi, M. and Pearce, J.M., 2023. Recycled Polycarbonate and Polycarbonate/Acrylonitrile Butadiene Styrene Feedstocks for Circular Economy Product Applications with Fused Granular Fabrication-Based Additive Manufacturing. Sustainable Materials and Technologies, Vol 38, e00730. DOI: 10.1016/j.susmat.2023.e00730

  2. Romani, A., Levi, M. and Pearce, J.M., 2023. Recycled Polycarbonate and Polycarbonate/Acrylonitrile Butadiene Styrene Feedstocks for Circular Economy Product Applications with Fused Granular Fabrication-Based Additive Manufacturing. Sustainable Materials and Technologies, Vol 38, e00730. DOI: 10.1016/j.susmat.2023.e00730

  3. Romani, A., Levi, M. and Pearce, J.M., 2023. Recycled Polycarbonate and Polycarbonate/Acrylonitrile Butadiene Styrene Feedstocks for Circular Economy Product Applications with Fused Granular Fabrication-Based Additive Manufacturing. Preprint. Available at SSRN. DOI: 10.2139/ssrn.4508039

  4. Pearce, J.M., Romani, A. 2023. Designs for Recycled PC and PC-ABS feedstock project. Project repository. Available at OSF.io. Link: https://osf.io/z9fnk/

  5. Pearce, J.M., Romani, A. 2023. GigabotX improvements. Project repository. Available at OSF.io. Link: https://osf.io/gxuqf/